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I joined NFCU yesterday. I love them! I did a lot of research on credit unions and they are easily one of the top CU's out there.
I only have an account with one credit union right now: DCU. And so far, I've been very happy with them. Unfortunately, they turned me down for a CC in 2013, but I'm still interested in getting one from them in the not too distant future (I still kept the savings and checking accounts when they turned me down for the CC).