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Now that I have "enough" available credit, I would still like to convert some of the credit which is less useful to me into the kind of credit I find more useful, namely credit union platinum non-rewards cards, and personal lines of credit.
Will I benefit from preemptively closing or reducing limits on the less useful accounts?
It could if your current total limits/exposure coud potentially be the constraint to approval/growth of the products that you desire. Whether or not that is the case would no doubt be lender-specific and almost impossible to determine under most circumstances.